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4-a- The "wandering" of the specific heat jump |
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Our calorimetry measurements have revealed a series of unexpected behaviours along the transition line separating the metal from the magnetic quantised phases: -1- The specific heat jump at the metal-FISDW transition, for low magnetic fields, is comparable with the value predicted by the BCS model of superconductivity [1] (weak coupling), while for strong fields the jump rises toward a very strong coupling (beyond that of lead) (Fig. 1).
-2- The jump at the transition oscillates along the quantised FISDW phases (Fig. 2). This result initiated a theoretical calculation in the framework of the "quantised nesting" model [2]. For strong fields, the jump rises to a "strong coupling" value that is NOT explained by the available theoretical models.
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-3- Our simultaneous specific heat and thermal conductivity measurements provided spectacular information about these critical phenomena. Fixed field specific heat measurements indicate the presence of two successive transitions (Fig. 3). Thermal conductivity strangely displays that only one of them exhibits a noticeable anomaly: the lowest temperature one. This difference in criticality behaviour is not explained.
-4- In strong fields, close to the "strong coupling" jump, other phenomena are revealed: two specific heat jumps of same amplitude may yield very different thermal conductivity anomalies, whereas symmetrically two very different jumps may give rise to similar amplitude anomalies [publi 21]. The magnetocaloric effect (see the following) leads in the same field range to an irreversible behaviour, while the effect is reversible on crossing the low field phase transitions [publi 8]. |
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Organic conductors
(4/8)
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