Tuning dimensionality, magnetism and conduction in van-der-Waals Mott insulators TMPS

Matthew Coak , University of Birmingham

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The van-der-Waals antiferromagnets TMPS3, where TM = Transition Metal, form an ideal playground for tuning both low-dimensional magnetic and electronic properties [1-4]. These are layered honeycomb antiferromagnetic Mott insulators, long studied as near-ideal 2D magnetic systems with a rich landscape of competing interactions and a variety of magnetic properties across the family.